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Optimal Dynamic Discrimination of Similar Molecules Through Quantum Learning Control

hal.structure.identifier
dc.contributor.authorRabitz, Herschel*
hal.structure.identifier
dc.contributor.authorRamakhrishna, Viswanath*
hal.structure.identifierCEntre de REcherches en MAthématiques de la DEcision [CEREMADE]
dc.contributor.authorTurinici, Gabriel
HAL ID: 16
ORCID: 0000-0003-2713-006X		*
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dc.contributor.authorLi, Baiqing*
dc.date.accessioned2012-09-04T08:13:17Z
dc.date.available2012-09-04T08:13:17Z
dc.date.issued2002
dc.identifier.urihttps://basepub.dauphine.fr/handle/123456789/9885
dc.language.isoenen
dc.subjectquantum systemsen
dc.subjectoptimal dynamic discriminationen
dc.subjectoptimal controlen
dc.subject.ddc520en
dc.titleOptimal Dynamic Discrimination of Similar Molecules Through Quantum Learning Controlen
dc.typeArticle accepté pour publication ou publié
dc.contributor.editoruniversityotherChemistry Department http://www.princeton.edu/chemistry/index.xml Princeton University;États-Unis
dc.description.abstractenA paradigm for discriminating similar quantum systems in the laboratory is presented based on optimal control principles with the aid of closed loop learning algorithms. The optimal dynamic discrimination (ODD) process is simulated for a noninteracting mixture of up to three similar finite-dimensional quantum systems. The optimal control field giving rise to species discrimination, that considers the presence of field and observation noise, is deduced with a genetic algorithm (GA). The similar quantum systems yield distinct dynamics and detection signals, although influenced by the same control laser pulse. The ODD process is shown to operate by drawing on constructive and destructive interference effects to simultaneously maximize or minimize the signals from each of the species in the mixture. The ODD technique may have applications to the analysis and separation of possibly even complex chemical species.en
dc.relation.isversionofjnlnameThe Journal of Physical Chemistry. B
dc.relation.isversionofjnlvol106en
dc.relation.isversionofjnlissue33en
dc.relation.isversionofjnldate2002
dc.relation.isversionofjnlpages8125-8131en
dc.relation.isversionofdoihttp://dx.doi.org/10.1021/jp0204657en
dc.relation.isversionofjnlpublisherACPen
dc.subject.ddclabelSciences connexes (physique, astrophysique)en
dc.relation.forthcomingnonen
dc.relation.forthcomingprintnonen
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